Highly efficient one-pot/one-step synthesis of multiblock copolymers from three-component polymerization of carbon dioxide, epoxide and lactone

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Highly efficient one-pot/one-step synthesis of multiblock copolymers from three-component polymerization of carbon dioxide, epoxide and lactone† †Electronic supplementary information (ESI) available: Text, figures and tables giving general experimental procedures and characterization data for multiblock copolymers. See DOI: 10.1039/c4sc03593c Click here for additional data file.

It is a long-standing challenge to combine mixed monomers into multiblock copolymer (MBC) in a onepot/one-step polymerization manner. We report the first example of MBC with biodegradable polycarbonate and polyester blocks that were synthesized from highly efficient one-pot/one-step polymerization of cyclohexene oxide (CHO), CO2 and 3-caprolactone (3-CL) in the presence of zinc– cobalt double m...

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ژورنال

عنوان ژورنال: Chemical Science

سال: 2015

ISSN: 2041-6520,2041-6539

DOI: 10.1039/c4sc03593c